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@ednadolski's photos look tremendous, so I think I might be splitting hairs here.
But his close up shot shows the sanded grout to be exactly what it is: rounded translucent quartz grains. Those look nothing like real ballast that is angular and opaque. Perhaps the size and color is all the really matters and his sieving of the grout definitely refines the look.
It's interesting. That quartz look issue is the same issue I have with the Scenic Express stuff I've been trying out. I don't remember it being a problem on my last layout though. It's interesting. I think it looks really good in this photo.https://imgur.com/dDKiYpw.jpgBut not here.https://imgur.com/9WSwMqV.jpgI'm starting to think it's all about the angle you view it at.
This is an example of a more ballast-looking material on @GaryHinshaw's TBC https://www.therailwire.net/forum/index.php?topic=24108.msg325821#msg325821. I couldn't find where it was sourced from (despite Gary's very helpful index on his thread!) but this material is clearly rock and not a grain of quartz in sight. I would guess limestone.
Limestone screenings are pretty common at landscaping places, at least where I've lived. They also sell it as a soil amendment in a finer form but I am not sure how fine it really is.
Unless you find something that is mostly fines/dust, I'd suspect that the vast majority of it would be far too large to use as ballast.Ed