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This is the place you want! They cater to machine shops, so their bits have a larger chuck that work great in pin vices. Plus, they’re cheap!https://www.drillbitsunlimited.com/
I am looking to purchase some small diameter drill bits in sizes from 60-80. I had a set I purchased from Micro-Mark years ago, but many have broken over time. I was wondering if there is a particular set that anyone could recommend that would last a long time. I don't mind paying a little extra for a better set.
Those are 1/8" shank Tungsten Carbide (TC) drills used for drilling PC boards. They also have split-shank points, and will cut through most materials like through butter. Extremely sharp, hard, and very fragile. I use TC bits very often, but they break very easily when drilling by hand. I usually use them iin a drill press. For hand drilling (in pin vise) regular High Speed Steel drill bits are much more robust.
If you decide to go carbide, these prices cannot be beaten for a pack of ten in a protective case:https://www.ebay.com/itm/10Pcs-1-8-Shank-Spiral-Flute-Tungsten-Carbide-Micro-PCB-Drill-Bit-0-2-0-9mm-Tip-/262902302178?var=&hash=item3d3632c5e2Sometimes, on the smaller diameter bits I break the bit off leaving about 1/8' and "resharpen" it using my cutoff disc, holding the bit at ~60 degress to the disc while rotating. This makes the bit less prone to breakage (less deflection) during hand drilling.It really does not matter if the sharpening is perfect, but try to get the resultant point in the center of the bit.